You can create a dual winxp boot. You can make an account (users control panel) log into it and turn off all the extras and run explorer in *minimal* mode. You could also create a custom boot account (safe mode type boot) that you select when starting up that loads only the bare minimum services you need.
Your best option is to create an account with just your games loaded on that account running windows in minimal mode (no fancy bars, effects, etc.) and turn off any start-up programs that aren't vital to your gaming experience. (anti-virus, montoring software, communications software, etc.). Although it's been my experience that doing all these thing just won't dramatically improve any hardware performance to go through all the trouble of loggin in and out of accounts or setting up a dual boot system.
System maintenence is going to get you the best performance as tarun mentioned.
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